Development of pure silica cha membranes for co2 separation

Daishi Takayama, Katsunori Ishii, Mikihiro Nomura, Takamasa Onoki, Takuya Okuno, Hiromasa Tawarayama, Shinji Ishikawa

Research output: Contribution to journalArticlepeer-review

2 Citations (Scopus)

Abstract

Thin pure-silica chabazite (Si-CHA) membranes have been synthesized by using a secondary growth method on a porous silica substrate. A CO2 permeance of 2.62 × 10−6 mol m−2 s−1 Pa−1 with a CO2/CH4 permeance ratio of 62 was obtained through a Si-CHA membrane crystallized for 8 h using a parent gel of H2O/SiO2 ratio of 4.6. The CO2 permeance through the Si-CHA membrane on a porous silica substrate was twice as high as that through the membrane synthesized on a porous alumina substrate, which displayed a similar zeolite layer thickness.

Original languageEnglish
Article number926
JournalMembranes
Volume11
Issue number12
DOIs
Publication statusPublished - 2021 Dec

Keywords

  • CO separation
  • Inorganic membrane
  • Membrane separation
  • Pure silica CHA-type zeolite
  • Silica substrates
  • Zeolite

ASJC Scopus subject areas

  • Chemical Engineering (miscellaneous)
  • Process Chemistry and Technology
  • Filtration and Separation

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