Abstract
Second-order nonlinear optical effects, a linear electro-optic (EO) effect and optical rectification (OR), were observed in surface immobilized gold nanospheres (SIGNs) above a gold surface with a gap of about 1.4 nm. The EO and OR measurements were performed in an attenuated total reflection geometry under a surface plasmon resonance condition. While it has been reported that the SIGN structure shows considerable second-harmonic generation activity, there has been no report on a linear EO effect and OR in the SIGN structure. The effective second-order susceptibilities of a single SIGN structure were evaluated to be 13 pm V-1 (EO) and 40 pmV-1 (OR). Although the theory predicts that the susceptibilities of EO and OR will be equal, the observed susceptibilities were different. The reasons for this discrepancy are discussed.
| Original language | English |
|---|---|
| Article number | 495101 |
| Journal | Journal of Physics D: Applied Physics |
| Volume | 43 |
| Issue number | 49 |
| DOIs | |
| Publication status | Published - 2010 Dec 15 |
| Externally published | Yes |
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ASJC Scopus subject areas
- Condensed Matter Physics
- Electronic, Optical and Magnetic Materials
- Acoustics and Ultrasonics
- Surfaces, Coatings and Films
Cite this
Electro-optic effect and optical rectification in gold nanoparticles immobilized above a gold surface. / Uchiho, Yuichi; Shimojo, Masayuki; Kajikawa, Kotaro.
In: Journal of Physics D: Applied Physics, Vol. 43, No. 49, 495101, 15.12.2010.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - Electro-optic effect and optical rectification in gold nanoparticles immobilized above a gold surface
AU - Uchiho, Yuichi
AU - Shimojo, Masayuki
AU - Kajikawa, Kotaro
PY - 2010/12/15
Y1 - 2010/12/15
N2 - Second-order nonlinear optical effects, a linear electro-optic (EO) effect and optical rectification (OR), were observed in surface immobilized gold nanospheres (SIGNs) above a gold surface with a gap of about 1.4 nm. The EO and OR measurements were performed in an attenuated total reflection geometry under a surface plasmon resonance condition. While it has been reported that the SIGN structure shows considerable second-harmonic generation activity, there has been no report on a linear EO effect and OR in the SIGN structure. The effective second-order susceptibilities of a single SIGN structure were evaluated to be 13 pm V-1 (EO) and 40 pmV-1 (OR). Although the theory predicts that the susceptibilities of EO and OR will be equal, the observed susceptibilities were different. The reasons for this discrepancy are discussed.
AB - Second-order nonlinear optical effects, a linear electro-optic (EO) effect and optical rectification (OR), were observed in surface immobilized gold nanospheres (SIGNs) above a gold surface with a gap of about 1.4 nm. The EO and OR measurements were performed in an attenuated total reflection geometry under a surface plasmon resonance condition. While it has been reported that the SIGN structure shows considerable second-harmonic generation activity, there has been no report on a linear EO effect and OR in the SIGN structure. The effective second-order susceptibilities of a single SIGN structure were evaluated to be 13 pm V-1 (EO) and 40 pmV-1 (OR). Although the theory predicts that the susceptibilities of EO and OR will be equal, the observed susceptibilities were different. The reasons for this discrepancy are discussed.
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UR - http://www.scopus.com/inward/citedby.url?scp=78650097572&partnerID=8YFLogxK
U2 - 10.1088/0022-3727/43/49/495101
DO - 10.1088/0022-3727/43/49/495101
M3 - Article
AN - SCOPUS:78650097572
VL - 43
JO - Journal Physics D: Applied Physics
JF - Journal Physics D: Applied Physics
SN - 0022-3727
IS - 49
M1 - 495101
ER -