Spin fluctuations in the spin-1/2 kagome lattice antiferromagnet (Rb1-xCsx)2Cu3SnF12 around the quantum critical point detected by muon spin relaxation technique

Takao Suzuki, Kazuya Katayama, Ikuto Kawasaki, Isao Watanabe, Hidekazu Tanaka

Research output: Contribution to journalArticle

Abstract

Zero- and longitudinal-field muon spin relaxation (ZF-, LF-μSR) measurements were carried out on the spin-1/2 kagome lattice antiferromagnet (Rb1-xCsx)2Cu3SnF12 with x = 0.53 and 0.6, where xc = 0.53 is the quantum critical point between the antiferromagnetically ordered phase and the valence-bond-glass phase. In the case of xc = 0.53, the muon spin relaxation rate at LF 200 gauss increases monotonically with decreasing temperature and shows no evidence for a magnetic order. The LF dependence of the muon spin relaxation rate, which corresponds to the fluctuating frequency spectrum, shows "white" spectrum behavior down to 0.3 K. These results indicate that internal magnetic fields fluctuate and are consistent with reported results of magnetic susceptibility measurement for xc = 0.53. In the case of x = 0.60, which is adjacent to the quantum critical point, the partial missing asymmetry in ZF-μSR time spectra is observed from a higher temperature than the antiferromagnetic phase transition temperature. It is suggested that large spin fluctuations peculiar to the quantum critical region appear.

Original languageEnglish
Article number074708
JournalJournal of the Physical Society of Japan
Volume87
Issue number7
DOIs
Publication statusPublished - 2018 Jan 1

Fingerprint

muons
critical point
transition temperature
asymmetry
valence
magnetic permeability
glass
magnetic fields
temperature

ASJC Scopus subject areas

  • Physics and Astronomy(all)

Cite this

Spin fluctuations in the spin-1/2 kagome lattice antiferromagnet (Rb1-xCsx)2Cu3SnF12 around the quantum critical point detected by muon spin relaxation technique. / Suzuki, Takao; Katayama, Kazuya; Kawasaki, Ikuto; Watanabe, Isao; Tanaka, Hidekazu.

In: Journal of the Physical Society of Japan, Vol. 87, No. 7, 074708, 01.01.2018.

Research output: Contribution to journalArticle

@article{b0cfe6330389477f9ecb4658e971fb2b,
title = "Spin fluctuations in the spin-1/2 kagome lattice antiferromagnet (Rb1-xCsx)2Cu3SnF12 around the quantum critical point detected by muon spin relaxation technique",
abstract = "Zero- and longitudinal-field muon spin relaxation (ZF-, LF-μSR) measurements were carried out on the spin-1/2 kagome lattice antiferromagnet (Rb1-xCsx)2Cu3SnF12 with x = 0.53 and 0.6, where xc = 0.53 is the quantum critical point between the antiferromagnetically ordered phase and the valence-bond-glass phase. In the case of xc = 0.53, the muon spin relaxation rate at LF 200 gauss increases monotonically with decreasing temperature and shows no evidence for a magnetic order. The LF dependence of the muon spin relaxation rate, which corresponds to the fluctuating frequency spectrum, shows {"}white{"} spectrum behavior down to 0.3 K. These results indicate that internal magnetic fields fluctuate and are consistent with reported results of magnetic susceptibility measurement for xc = 0.53. In the case of x = 0.60, which is adjacent to the quantum critical point, the partial missing asymmetry in ZF-μSR time spectra is observed from a higher temperature than the antiferromagnetic phase transition temperature. It is suggested that large spin fluctuations peculiar to the quantum critical region appear.",
author = "Takao Suzuki and Kazuya Katayama and Ikuto Kawasaki and Isao Watanabe and Hidekazu Tanaka",
year = "2018",
month = "1",
day = "1",
doi = "10.7566/JPSJ.87.074708",
language = "English",
volume = "87",
journal = "Journal of the Physical Society of Japan",
issn = "0031-9015",
publisher = "Physical Society of Japan",
number = "7",

}

TY - JOUR

T1 - Spin fluctuations in the spin-1/2 kagome lattice antiferromagnet (Rb1-xCsx)2Cu3SnF12 around the quantum critical point detected by muon spin relaxation technique

AU - Suzuki, Takao

AU - Katayama, Kazuya

AU - Kawasaki, Ikuto

AU - Watanabe, Isao

AU - Tanaka, Hidekazu

PY - 2018/1/1

Y1 - 2018/1/1

N2 - Zero- and longitudinal-field muon spin relaxation (ZF-, LF-μSR) measurements were carried out on the spin-1/2 kagome lattice antiferromagnet (Rb1-xCsx)2Cu3SnF12 with x = 0.53 and 0.6, where xc = 0.53 is the quantum critical point between the antiferromagnetically ordered phase and the valence-bond-glass phase. In the case of xc = 0.53, the muon spin relaxation rate at LF 200 gauss increases monotonically with decreasing temperature and shows no evidence for a magnetic order. The LF dependence of the muon spin relaxation rate, which corresponds to the fluctuating frequency spectrum, shows "white" spectrum behavior down to 0.3 K. These results indicate that internal magnetic fields fluctuate and are consistent with reported results of magnetic susceptibility measurement for xc = 0.53. In the case of x = 0.60, which is adjacent to the quantum critical point, the partial missing asymmetry in ZF-μSR time spectra is observed from a higher temperature than the antiferromagnetic phase transition temperature. It is suggested that large spin fluctuations peculiar to the quantum critical region appear.

AB - Zero- and longitudinal-field muon spin relaxation (ZF-, LF-μSR) measurements were carried out on the spin-1/2 kagome lattice antiferromagnet (Rb1-xCsx)2Cu3SnF12 with x = 0.53 and 0.6, where xc = 0.53 is the quantum critical point between the antiferromagnetically ordered phase and the valence-bond-glass phase. In the case of xc = 0.53, the muon spin relaxation rate at LF 200 gauss increases monotonically with decreasing temperature and shows no evidence for a magnetic order. The LF dependence of the muon spin relaxation rate, which corresponds to the fluctuating frequency spectrum, shows "white" spectrum behavior down to 0.3 K. These results indicate that internal magnetic fields fluctuate and are consistent with reported results of magnetic susceptibility measurement for xc = 0.53. In the case of x = 0.60, which is adjacent to the quantum critical point, the partial missing asymmetry in ZF-μSR time spectra is observed from a higher temperature than the antiferromagnetic phase transition temperature. It is suggested that large spin fluctuations peculiar to the quantum critical region appear.

UR - http://www.scopus.com/inward/record.url?scp=85049659635&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=85049659635&partnerID=8YFLogxK

U2 - 10.7566/JPSJ.87.074708

DO - 10.7566/JPSJ.87.074708

M3 - Article

VL - 87

JO - Journal of the Physical Society of Japan

JF - Journal of the Physical Society of Japan

SN - 0031-9015

IS - 7

M1 - 074708

ER -